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Blar i University of Bergen Library på tidsskrift "ACS Catalysis"

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    • Challenging Metathesis Catalysts with Nucleophiles and Brønsted Base: Examining the Stability of State-of-the-Art Ruthenium Carbene Catalysts to Attack by Amines 

      do Nascimento, Daniel Luis; Reim, Immanuel; Foscato, Marco; Jensen, Vidar Remi; Fogg, Deryn Elizabeth (Journal article; Peer reviewed, 2020)
      Critical to advancing the uptake of olefin metathesis in leadingcontexts, including pharmaceutical manufacturing, is identification of highlyactive catalysts that resist decomposition. Amines constitute an aggressivechallenge ...
    • Ethylene-Triggered Formation of Ruthenium Alkylidene from Decomposed Catalyst 

      Smit, Wietse; Foscato, Marco; Occhipinti, Giovanni; Jensen, Vidar Remi (Journal article; Peer reviewed, 2020)
      Ethylene is known to readily decompose ruthenium-based olefin metathesis catalysts, such as Grubbs second-generation catalyst (GII), by forming the unsubstituted ruthenacyclobutane (Ru-2) that may undergo a 1,2-H shift and ...
    • The Impact of Water on Ru-Catalyzed Olefin Metathesis: Potent Deactivating Effects Even at Low Water Concentrations 

      Blanco, Christian O.; Sims, Joshua; Nascimento, Daniel L.; Goudreault, Alexandre Y.; Steinmann, Stephan N.; Michel, Carine; Fogg, Deryn Elizabeth (Journal article; Peer reviewed, 2021)
      Ruthenium catalysts for olefin metathesis are widely viewed as water-tolerant. Evidence is presented, however, that even low concentrations of water cause catalyst decomposition, severely degrading yields. Of 11 catalysts ...

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