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dc.contributor.authorHuq, Farhana
dc.contributor.authorSmalley, P. Craig
dc.contributor.authorMørkved, Pål Tore
dc.contributor.authorJohansen, Ingar
dc.contributor.authorYarushina, Viktoriya
dc.contributor.authorJohansen, Harald
dc.date.accessioned2018-04-27T12:23:20Z
dc.date.available2018-04-27T12:23:20Z
dc.date.issued2017-08
dc.PublishedHuq F, Smalley, Mørkved PT, Johansen I, Yarushina V, Johansen H. The Longyearbyen CO2 Lab: Fluid communication in reservoir and caprock. International Journal of Greenhouse Gas Control. 2017;63:59-76eng
dc.identifier.issn1750-5836en_US
dc.identifier.issn1878-0148en_US
dc.identifier.urihttps://hdl.handle.net/1956/17671
dc.description.abstractThe Longyearbyen CO2 Lab of Svalbard, Norway was established to estimate the potential for geological carbon sequestration at Spitsbergen. Several monitoring wells were drilled in and around the planned CO2 injection site. These revealed a Triassic to Cretaceous stratigraphy consisting of (from top to bottom) a zone of permafrost, the aquifer, the caprock shale, and the upper, middle and lower reservoir. This paper uses two tools to investigate fluid communication within and between these entities: 87Sr/86Sr of formation waters extracted from cores using the residual salt analysis (RSA) method, and the δ13C of gases, principally methane and CO2, degassed from core samples. The Sr RSA data reveal that the upper reservoir rocks have very constant formation water 87Sr/86Sr (0.7130) in wells several kilometres apart, suggesting good lateral communication on a geological timescale. However, there is a distinct barrier to vertical communication within the middle reservoir, indicated by a step change in 87Sr/86Sr (0.7130–0.7112), corresponding to thin but presumably laterally extensive (>1.5 km) lagoonal mudrocks. The aquifer, which shows a gradient in 87Sr/86Sr, is also interpreted to have some degree of vertical internal communication on a geological time scale. The caprock shale shows large-scale (over 350 m) smooth vertical gradient in 87Sr/86Sr (0.7200-0.7130). This is indicative of an ongoing mixing process between high- 87Sr/86Sr waters within the caprock and lower- 87Sr/86Sr waters in the underlying reservoir. Diffusion and flow modelling of the Sr data suggest that at some time in the past, shale fluid transport properties were enhanced by the formation of temporary pressure escape features (fractures or chimneys) during deep burial and uplift, or cycles of glaciation. Nevertheless, the smooth compositional gradient in the caprock indicates that fluid mixing has subsequently taken place slowly, dominated by diffusion. This interpretation is supported by the gas isotope data, where systematic variations in gas δ13C (-50‰ to −32‰) values also indicate slow and incomplete diffusional fluid mixing. These are positive indicators for caprock effectiveness during a CO2 injection project.en_US
dc.language.isoengeng
dc.publisherElsevieren_US
dc.rightsAttribution CC BY-NC-ND
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/
dc.subjectCO2 storageeng
dc.subjectSr isotopeeng
dc.subjectC isotopeeng
dc.subjectSite characterizationeng
dc.subjectFluid floweng
dc.subjectLarge-scale CCSeng
dc.subjectCaprockeng
dc.titleThe Longyearbyen CO2 Lab: Fluid communication in reservoir and caprocken_US
dc.typePeer reviewed
dc.typeJournal article
dc.date.updated2017-12-20T09:27:40Z
dc.description.versionacceptedVersionen_US
dc.rights.holderCopyright 2017 Elsevier Ltd. All rights reserved.en_US
dc.identifier.doihttps://doi.org/10.1016/j.ijggc.2017.05.005
dc.identifier.cristin1485231
dc.source.journalInternational Journal of Greenhouse Gas Control
dc.source.pagenumber59-76
dc.identifier.citationInternational Journal of Greenhouse Gas Control. 2017;63:59-76
dc.source.volume63


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